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• W3208296645 endingPage "12297" @default.
• W3208296645 startingPage "12290" @default.
• W3208296645 abstract "The degeneration of organic–inorganic hybrid perovskite solar cells (PSCs) under ambient air is a serious challenge that prevents the commercialization of PSCs. The introduction of hydrophobic long-chain organic cations into the perovskite film is a promising way to improve the long-term stability of devices. However, this approach always comes with the sacrifice of the power conversion efficiency (PCE). In this work, we introduce a novel one-step double ion passivation route together using phenylethylamine ion (PEA+) and SCN– to passivate the grain boundary and surface of the perovskite polycrystalline film by crystal engineering to fabricate all air-processed, stable PSCs. Compared with three-dimensional (3D) MAPbI3 perovskite films, the PEA+ and SCN– codoped MAPbI3 perovskite films from the single crystal engineering have a larger grain size and better stability with a longer carrier lifetime and lower electron trap state density. The champion PCE of 18.04% with negligible hysteresis was achieved for the 0.05 M PEA+ and SCN– codoped PSCs, which exhibit 25% higher efficiency than the MAPbI3 solar cell fabricated using the traditional precursor solution mixing method. The devices without encapsulation still maintain 82% of their original PCE when stored over 750 h under ambient air conditions with a relative humidity of 50%." @default.
• W3208296645 created "2021-11-08" @default.
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• W3208296645 date "2021-10-20" @default.
• W3208296645 modified "2023-10-14" @default.
• W3208296645 title "Interface and Grain Boundary Passivation by PEA-SCN Double Ions via One-Step Crystal Engineering for All Air-Processed, Stable Perovskite Solar Cells" @default.
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• W3208296645 doi "https://doi.org/10.1021/acsaem.1c02113" @default.
• W3208296645 hasPublicationYear "2021" @default.
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