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• W3208460461 abstract "Direct conversion of CO2 into chemical compounds has become a prospective pathway to transform CO2 into valuable chemical compounds. The introduction of porous materials with high uptake into photocatalytic systems can enrich the CO2 absorption on the surface of the photocatalyst for catalytic conversion. In this regard, another feasible strategy can be accomplished via combining commercial photocatalyst materials with porous supporting materials. The present study investigated a series of ZnO-incorporated ZSM-5 catalysts to produce solar fuels under UV–visible light irradiation. ZnO/ZSM-5 was synthesized using the wet impregnation method using Zn(CH3COO)2 as a reagent, followed by calcination. Various characterizations were also conducted to study morphology, structure, absorbance, and physiochemical properties of the photocatalysts. SEM-EDX images showed that ZnO was successfully incorporated into ZSM-5 surfaces with a particle size of around 50 nm. The optical properties of ZnO/ZSM-5 correspond to 3.36 eV, showing an increase in the bandgap value compared to pure ZnO, with 3.18 eV. The solar fuel production, including formic acid (HCOOH), formaldehyde (HCOH), and methanol (CH3OH) evolution was evaluated under UV–visible light irradiation. The designed composite ZnO/ZSM-5 catalyst achieved methanol and formic acid yields of 39.2 µmol/g·h and 0.72 µmol/g·h µmol/(g·h), respectively, which are about 1.5- and 2.5-fold higher than the neat ZnO catalyst. The improved yield and selectivity towards methanol products are attributed to the greater light absorption, more efficient charge transfer, nanostructure morphology, and more active sites available for CO2 adsorption." @default.
• W3208460461 created "2021-11-08" @default.
• W3208460461 creator A5036754998 @default.
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• W3208460461 date "2021-10-20" @default.
• W3208460461 modified "2023-09-25" @default.
• W3208460461 title "ZnO-Incorporated ZSM-5 for Photocatalytic CO2 Reduction into Solar Fuels under UV–Visible Light" @default.
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• W3208460461 doi "https://doi.org/10.3390/eccs2021-11205" @default.
• W3208460461 hasPublicationYear "2021" @default.
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