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• W3208490640 endingPage "1246" @default.
• W3208490640 startingPage "1238" @default.
• W3208490640 abstract "Herein, spherical hollow N-doped carbon-incorporated UiO-66 metal-organic frameworks (MOF, H-UiO-66) are synthesized using bio-inspired polydopamine (pDA) nanoparticles as multifunctional starting templates. The calculated band properties (ECB = -0.45 eV and EVB = 2.05 eV versus normal hydrogen electrode (NHE)) strongly reveals the visible light absorption of H-UiO-66 nanostructures thanks to the spherical shape-defined morphology as well as cavity of the hollow structure. The evaluation of photoelectrochemical (PEC) water splitting performance of H-UiO-66 photoanodes shows maximum photocurrent density as 10.95 mA/cm2 at 1.53 V versus RHE under LED illumination in which almost no response is recorded at dark. Furthermore, the improved visible-light sensitive PEC water splitting performance of H-UiO-66 photoanodes could be attributed to the main advantages of the one-pot synthesis method of hollow MOFs using multifunctional pDA as follows: i) the hollow morphology provides superior incident photon scattering and multi-reflection of photons inside the MOF cavity; ii) presence of N-doped carbon incorporated morphology facilitates the absorption of water molecules as well as the π-polar interaction between water and carbon; and iii) the reduced bang-gap led to the optical localization of light within H-UiO-66 clusters, suggesting a new generation of heterogeneous well-defined nanostructures for sustainable PEC hydrogen production." @default.
• W3208490640 created "2021-11-08" @default.
• W3208490640 creator A5040382756 @default.
• W3208490640 creator A5058071262 @default.
• W3208490640 creator A5077675879 @default.
• W3208490640 date "2022-02-01" @default.
• W3208490640 modified "2023-10-12" @default.
• W3208490640 title "Spherical shape-defined hollow UiO-66 metal-organic frameworks with superior incident photon scattering for enhanced photoelectrochemical H2 evolution" @default.
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• W3208490640 doi "https://doi.org/10.1016/j.jcis.2021.10.145" @default.
• W3208490640 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34739987" @default.
• W3208490640 hasPublicationYear "2022" @default.
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