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• W3208498178 abstract "Silicon (Si) is an auspicious anode material in next-generation lithium-ion batteries due to its exceptional theoretical gravimetric capacity, environmental friendliness, and high natural abundance. However, the practical application of Si anodes remains a must-solve challenge because of its drastic capacity fading that results from the inherent property of drastic volume expansion of Si during repeated lithiation and delithiation. Developing binders employed in robust electrodes has been considered an economical and practical method to affect the electrochemical performance of Si-based electrodes. Some natural polymers have demonstrated good adhesive properties with Si-active materials. However, they have limited capacity to keep the structural integrity of electrodes because the network structures solely based on weak hydrogen bonds are susceptible to deformation during cycling. Herein, we develop an in situ covalently cross-linked three-dimensional (3D) supramolecular network and apply it to the Si electrode to improve cycling performance. This network architecture is constructed using furan-modified branched arabinoxylan of corn fiber gum (CFG) and an ionically conductive cross-linker of maleimido-poly(ethylene glycol) (PEG) through the Diels-Alder reaction. The maleimide groups in PEG can react spontaneously with the furan groups in CFG at room temperature without any other stimulation, thus forming strong covalent bonds in the network. The cross-linked CFG-PEG binder has demonstrated robust adhesive properties with Si-active materials and the current collector. The branching of CFG and functional groups of PEG are conducive to improving the lithium-ion conductivity in the silicon anode, resulting in excellent rate performances. The Si anode with a cross-linked CFG-PEG binder exhibits superior cycling stability. As a result, an in situ cross-linking 3D network as a novel binder has a great potential for fabricating an advanced Si anode in next-generation Li-ion batteries." @default.
• W3208498178 created "2021-11-08" @default.
• W3208498178 creator A5002189161 @default.
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• W3208498178 date "2021-11-03" @default.
• W3208498178 modified "2023-10-16" @default.
• W3208498178 title "In Situ Room-Temperature Cross-Linked Highly Branched Biopolymeric Binder Based on the Diels–Alder Reaction for High-Performance Silicon Anodes in Lithium-Ion Batteries" @default.
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• W3208498178 cites W1965297344 @default.
• W3208498178 cites W1984182988 @default.
• W3208498178 cites W1995165442 @default.
• W3208498178 cites W2009392360 @default.
• W3208498178 cites W2021172010 @default.
• W3208498178 cites W2022608115 @default.
• W3208498178 cites W2044390575 @default.
• W3208498178 cites W2047099464 @default.
• W3208498178 cites W2053703518 @default.
• W3208498178 cites W2061772853 @default.
• W3208498178 cites W2073994106 @default.
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• W3208498178 cites W2086608111 @default.
• W3208498178 cites W2112902557 @default.
• W3208498178 cites W2116735248 @default.
• W3208498178 cites W2124043346 @default.
• W3208498178 cites W2132253708 @default.
• W3208498178 cites W2133594054 @default.
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• W3208498178 cites W2238615125 @default.
• W3208498178 cites W2266225888 @default.
• W3208498178 cites W2317806057 @default.
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• W3208498178 cites W2345658523 @default.
• W3208498178 cites W2346234212 @default.
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• W3208498178 cites W2399966197 @default.
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• W3208498178 cites W2546966113 @default.
• W3208498178 cites W2550613263 @default.
• W3208498178 cites W2560125452 @default.
• W3208498178 cites W2560441782 @default.
• W3208498178 cites W2608197933 @default.
• W3208498178 cites W2737421643 @default.
• W3208498178 cites W2742065712 @default.
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• W3208498178 doi "https://doi.org/10.1021/acsami.1c16196" @default.
• W3208498178 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34727688" @default.
• W3208498178 hasPublicationYear "2021" @default.
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