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• W3208637871 endingPage "53903" @default.
• W3208637871 startingPage "53892" @default.
• W3208637871 abstract "On the premise of cleanliness and stability, improving the catalytic efficiency for the oxygen reduction reaction in the electrode reaction of fuel cells and metal-air batteries is of vital importance. Studies have shown that heteroatom doping and structural optimization are efficient strategies. Herein, a single-atom-like B-N3 configuration in carbon is designed for efficient oxygen reduction reaction catalysis inspired by the extensively studied transition metal M-Nx sites, which is supported on the ordered macroporous carbon prepared by utilizing a hydrogen-bonded organic framework as carbon and nitrogen sources and SiO2 spheres as a template. The co-doping of B/N and ordered macroporous structures promote the metal-free material high oxygen reduction catalytic performance in alkaline media. DFT calculations reveal that the B-N3 structure played a key role in enhancing the oxygen reduction activity by providing rich favorable *OOH and *OH adsorption sites on the B center. The promoted formation of *OH/*OOH intermediates accelerated the electrocatalyst reaction. This study provides new insights into the design of single-atom-like nonmetallic ORR electrocatalysts and synthesis of ordered macroporous carbons based on hydrogen-bonded organic frameworks." @default.
• W3208637871 created "2021-11-08" @default.
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• W3208637871 date "2021-11-05" @default.
• W3208637871 modified "2023-10-18" @default.
• W3208637871 title "Single-Atom-like B-N₃ Sites in Ordered Macroporous Carbon for Efficient Oxygen Reduction Reaction" @default.
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• W3208637871 doi "https://doi.org/10.1021/acsami.1c15661" @default.
• W3208637871 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34738781" @default.
• W3208637871 hasPublicationYear "2021" @default.
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