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- W3209302318 abstract "Diethylammonium nitrate, [N0 0 2 2][NO3], and its perdeuterated analogue, [N D D 2 2] [NO3], were structurally characterized and studied by infrared, Raman, and inelastic neutron scattering (INS) spectroscopy. Using these experimental data along with state-of-the-art computational materials modeling, we report unambiguous spectroscopic signatures of hydrogen-bonding interactions between the two counterions. An exhaustive assignment of the spectral features observed with each technique has been provided, and a number of distinct modes related to NH···O dynamics have been identified. We put a particular emphasis on a detailed interpretation of the high-resolution, broadband INS experiments. In particular, the INS data highlight the importance of conformational degrees of freedom within the alkyl chains, a ubiquitous feature of ionic liquid (IL) systems. These findings also enable an in-depth physicochemical understanding of protonic IL systems, a first and necessary step to the tailoring of hydrogen-bonding networks in this important class of materials." @default.
- W3209302318 created "2021-11-08" @default.
- W3209302318 creator A5000182813 @default.
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- W3209302318 creator A5085886271 @default.
- W3209302318 creator A5088152696 @default.
- W3209302318 date "2021-10-27" @default.
- W3209302318 modified "2023-10-13" @default.
- W3209302318 title "Spectroscopic Signatures of Hydrogen-Bonding Motifs in Protonic Ionic Liquid Systems: Insights from Diethylammonium Nitrate in the Solid State" @default.
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