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• W3209818420 abstract "Recent optical second-harmonic generation experiments observed unexpected broken spatial symmetries in the undoped spin-orbit Mott insulator ${mathrm{Sr}}_{2}{mathrm{IrO}}_{4}$, leading to intensive debates on the nature of its ground state. We propose that it is a canted antiferromagnetism (CAF) with a hidden order of circulating staggered pseudospin current. Symmetry analysis shows that a proper $c$-axis stacking of the CAF and the pseudospin current lead to a magnetoelectric coexistence state that breaks the twofold rotation, inversion, and time-reversal symmetries, consistent with experimental observations. We construct a three-dimensional Hubbard model with spin-orbit coupling and structural distortion for the five localized $5d$ Wannier orbitals centered at Ir sites and demonstrate the microscopic realization of the desired coexistence state in a wide range of band parameters via a combination of self-consistent Hartree-Fock and variational calculations." @default.
• W3209818420 created "2021-11-08" @default.
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• W3209818420 date "2021-10-27" @default.
• W3209818420 modified "2023-10-15" @default.
• W3209818420 title "Three-dimensional stacking of canted antiferromagnetism and pseudospin current in undoped Sr2IrO4 : Symmetry analysis and microscopic model realization" @default.
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• W3209818420 doi "https://doi.org/10.1103/physrevb.104.165145" @default.
• W3209818420 hasPublicationYear "2021" @default.
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