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• W3210100601 abstract "Lithium battery materials can be advantageously used for the selective sequestration of lithium ions from natural resources, which contain other cations in high excess. However, for practical applications, this new approach for lithium production requires the battery host materials to be stable over many cycles while retaining the high lithium selectivity. Here, a nearly symmetrical cell design was employed to show that LiFePO4 shows good capacity retention with cycling in artificial lithium brines representative of brines from Chile, Bolivia and Argentina. A quantitative correlation was identified between brine viscosity and capacity degradation, and for the first time it was demonstrated that the dilution of viscous brines with water significantly enhanced capacity retention and rate capability. The electrochemical and X-ray diffraction characterisation of the cycled electrodes also showed that the high lithium selectivity was preserved with cycling. Raman spectra of the cycled electrodes showed no signs of degradation of the carbon coating of LiFePO4, while scanning electron microscopy images showed signs of particle cracking, thus pointing towards interfacial reactions as the cause of capacity degradation." @default.
• W3210100601 created "2021-11-08" @default.
• W3210100601 creator A5027301994 @default.
• W3210100601 creator A5033741028 @default.
• W3210100601 creator A5035624765 @default.
• W3210100601 creator A5058236474 @default.
• W3210100601 date "2021-11-24" @default.
• W3210100601 modified "2023-09-27" @default.
• W3210100601 title "LiFePO ₄ Battery Material for the Production of Lithium from Brines: Effect of Brine Composition and Benefits of Dilution" @default.
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• W3210100601 doi "https://doi.org/10.1002/cssc.202102182" @default.
• W3210100601 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34730274" @default.
• W3210100601 hasPublicationYear "2021" @default.
• W3210100601 type Work @default.
• W3210100601 sameAs 3210100601 @default.

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