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- W3210109618 abstract "The photocatalytic reduction of CO2 to energy-rich chemicals is highly appealing for alleviation of energy crisis and environment pollution. The introduction of different active sites is a key factor to determine the reaction activity and selectivity. Here, we demonstrate the metal ion-dependent performance for photocatalytic CO2 reduction by anchoring transition metal ions (Co2+ and Ni2+) in an amine-functionalized boron imidazolate framework (BIF-43). As a result, [email protected]BIF-43 realized a high selectivity of 90.2% for the CO2-to-CO, while [email protected]BIF-43 achieved more efficient conversion with a high CO production rate of 2036.0 µmol g−1 h−1. Significantly, precise control of isolated metal site on a well-defined structure through coordination-assisted strategies enables us to better understand the specific effects of different metal-ion species on photoreduction of CO2 as well as the catalytic mechanism." @default.
- W3210109618 created "2021-11-08" @default.
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- W3210109618 date "2022-06-01" @default.
- W3210109618 modified "2023-10-09" @default.
- W3210109618 title "Anchoring metal ions in amine-functionalized boron imidazolate framework for photocatalytic reduction of CO2" @default.
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- W3210109618 doi "https://doi.org/10.1016/j.cclet.2021.10.061" @default.
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