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- W3210121745 abstract "A straightforward and divergent entry to α-fluorinated carbonyl and carboxyl derivatives is reported. Upon activation of amides with triflic anhydride and a 2-halo-pyridine and subsequent trapping of the resulting keteniminium ions with nucleophiles followed by a second electrophilic activation with NFSI and final hydrolysis, a range of amides can be transformed to α-fluorinated ketones, esters, and amides under mild conditions. Moreover, this reaction can be performed to yield enantioenriched products with a traceless chiral auxiliary." @default.
- W3210121745 created "2021-11-08" @default.
- W3210121745 creator A5003856165 @default.
- W3210121745 creator A5084905235 @default.
- W3210121745 date "2021-10-28" @default.
- W3210121745 modified "2023-10-03" @default.
- W3210121745 title "Divergent Synthesis of α-Fluorinated Carbonyl and Carboxyl Derivatives by Double Electrophilic Activation of Amides" @default.
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- W3210121745 doi "https://doi.org/10.1021/acs.orglett.1c03450" @default.
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