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- W3210726601 abstract "This work is the first report on a hole-selective tin-based perovskite solar cell (PSC) using the concept of a self-assembled monolayer (SAM) to modify the ITO surface to fabricate a uniform tin perovskite layer via a two-step sequential deposition method. Herein, we developed a preheating procedure to diminish effectively the amounts of hydroxyl groups and oxygen vacancies on the ITO surface to produce a uniform SAM. The ITO substrate preheated at 400 °C gave the best device performance for an efficiency of power conversion (PCE) reaching 6.5%, and 80% of the initial PCE was maintained in a glovebox for ∼1900 h. Electrochemical impedance spectra and time-resolved spectra were used to understand the interfacial charge recombination and hole-extraction kinetics in relation to the observed device performance. The present work thus provides a new direction for the development of SAM-based lead-free perovskite solar cells for their future scaled-up production." @default.
- W3210726601 created "2021-11-08" @default.
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- W3210726601 date "2021-11-03" @default.
- W3210726601 modified "2023-10-16" @default.
- W3210726601 title "Interfacial Engineering with a Hole-Selective Self-Assembled Monolayer for Tin Perovskite Solar Cells via a Two-Step Fabrication" @default.
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- W3210726601 doi "https://doi.org/10.1021/acsenergylett.1c02124" @default.
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