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• W3211174003 abstract "Ti3C2Tx, a member of the MXene, has attracted extensive interest because of its high conductivity, unique two-dimensional (2D) structure and intrinsic pseudocapacitance for supercapacitors. Flexible and freestanding Ti3C2Tx films are promising electrodes for functioned supercapacitors used in wearable and portable electronic devices. However, the severe self-restacking of 2D Ti3C2Tx nanosheets restraints their practical application. Herein, freestanding and flexible three-dimensional (3D) cross-linked Ti3C2Tx-Ca-SA (sodium alginate) films with expanded Ti3C2Tx interlayer spacing are reported. The expanded interlayer spacing allows more electrolyte ions to quickly intercalate providing more intercalation pseudocapacitance, while the 3D cross-linked microstructure ensures a continuous conductive network facilitating charges transport. Attributing to the unique structure, the Ti3C2Tx-Ca-SA film delivers an outstanding areal capacitance (633 mF cm-2 at 5 mV s-1). Meanwhile, the assembled all-solid-state pseudocapacitor shows good flexibility and capacity stability under various bending conditions. The device exhibits a high energy density up to 12.6 µWh cm-2 at the power density of 375 µW cm-2 and excellent cycling stability, which are much better than prior reported state-of-the-art supercapacitors. This research exploits a simple method to optimize the structure of MXene as state-of-the-art electrodes for high-performance flexible energy-storage devices." @default.
• W3211174003 created "2021-11-08" @default.
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• W3211174003 date "2022-03-01" @default.
• W3211174003 modified "2023-10-18" @default.
• W3211174003 title "3D Cross-linked Ti3C2Tx-Ca-SA films with expanded Ti3C2Tx interlayer spacing as freestanding electrode for all-solid-state flexible pseudocapacitor" @default.
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• W3211174003 doi "https://doi.org/10.1016/j.jcis.2021.10.127" @default.
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• W3211174003 hasPublicationYear "2022" @default.
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