Matches in SemOpenAlex for { <https://semopenalex.org/work/W3212257593> ?p ?o ?g. }
- W3212257593 abstract "Electronic states and their dynamics are of critical importance for electronic and optoelectronic applications. Here, various relevant electronic states in monolayer MoS2 , such as multiple excitonic Rydberg states and free-particle energy bands are probed with a high relative contrast of up to ≥200 via broadband (from ≈1.79 to 3.10 eV) static third-harmonic spectroscopy (THS), which is further supported by theoretical calculations. Moreover, transient THS is introduced to demonstrate that third-harmonic generation can be all-optically modulated with a modulation depth exceeding ≈94% at ≈2.18 eV, providing direct evidence of dominant carrier relaxation processes associated with carrier-exciton and carrier-phonon interactions. The results indicate that static and transient THS are not only promising techniques for the characterization of monolayer semiconductors and their heterostructures, but also a potential platform for disruptive photonic and optoelectronic applications, including all-optical modulation and imaging." @default.
- W3212257593 created "2021-11-22" @default.
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- W3212257593 date "2021-11-23" @default.
- W3212257593 modified "2023-10-18" @default.
- W3212257593 title "Probing Electronic States in Monolayer Semiconductors through Static and Transient Third‐Harmonic Spectroscopies" @default.
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- W3212257593 doi "https://doi.org/10.1002/adma.202107104" @default.
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