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• W3212858186 abstract "With the goal of maximizing the thermoelectric (TE) figure of merit $ZT$, Mahan and Sofo [Proc. Natl. Acad. Sci. USA 93, 7436 (1996)] found that the optimal transport distribution (TD) is a $ensuremath{delta}$ function. Materials, however, have TDs that appear to always be finite and nondiverging. Motivated by this observation, this study focuses on deriving what is the optimal bounded TD, which is determined to be a boxcar function for $ZT$ and a Heaviside function for power factor. From these optimal TDs, upper limits on $ZT$ and power factor are obtained; the maximum $ZT$ scales with ${mathrm{ensuremath{Sigma}}}_{mathrm{max}}T/{ensuremath{kappa}}_{l}$, where ${mathrm{ensuremath{Sigma}}}_{mathrm{max}}$ is the TD magnitude and ${ensuremath{kappa}}_{l}$ is the lattice thermal conductivity. These results help establish practical upper limits on the performance of TE materials and provide target TDs to guide band and/or scattering engineering strategies." @default.
• W3212858186 created "2021-11-22" @default.
• W3212858186 creator A5081691893 @default.
• W3212858186 date "2021-11-15" @default.
• W3212858186 modified "2023-10-16" @default.
• W3212858186 title "Limits of thermoelectric performance with a bounded transport distribution" @default.
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• W3212858186 doi "https://doi.org/10.1103/physrevb.104.184301" @default.
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