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- W3212865458 abstract "The nonradiative recombination of charge carriers at the hole transport layer (HTL)/perovskite interface generally induces remarkable performance loss of the inverted two-dimensional perovskite solar cells (2D PSCs). Herein, a cross-linkable small molecule of 2-mercaptoimidazole (2-MI) was introduced into the nickel oxide (NiOx)/2D perovskite interface. Experiments have confirmed the formation of Ni-N covalent bond by N atom in the 2-MI and Ni in the NiOx and the coordinating between S atom of 2-MI and under-coordinated Pb2+ near to the NiOx/perovskite interface, which contributes to creating a cross-linking between NiOx/perovskite interface to restrain charge carrier recombination and enhance the extraction of hole carriers at the interface. Besides, the 2-MI modification layer is also beneficial for promoting the crystallinity of 2D perovskite. Consequently, the inverted 2D PSCs with 2-MI modification achieved the best power conversion efficiency of 15%. This paves a route to acquire highly efficient 2D PSCs by constructing a cross-linking at the NiOx HTL/2D perovskite interface." @default.
- W3212865458 created "2021-11-22" @default.
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- W3212865458 date "2022-05-01" @default.
- W3212865458 modified "2023-09-23" @default.
- W3212865458 title "Small molecule interfacial cross-linker for highly efficient two-dimensional perovskite solar cells" @default.
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- W3212865458 doi "https://doi.org/10.1016/j.jechem.2021.10.026" @default.
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