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- W3213202893 endingPage "185" @default.
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- W3213202893 abstract "Natural systems drive the high-energy reactions of photosynthesis with efficient and broadband energy capture. Transition-metal photocatalysts similarly convert light into chemical reactivity, and yet suffer from light-limited operation and require blue-to-UV excitation. In photosynthesis, both light capture and reactivity have been optimized by separation into distinct sites. Inspired by this modular architecture, we synthesized a biohybrid photocatalyst by covalent attachment of the photosynthetic light-harvesting protein R-phycoerythrin (RPE) to the transition-metal photocatalyst tris(2,2′-bipyridine)ruthenium(II) ([Ru(bpy)3]2+). Spectroscopic investigation found that absorbed photoenergy was efficiently funneled from RPE to [Ru(bpy)3]2+. The utility of the biohybrid photocatalyst was demonstrated via an increase in yields for a thiol-ene coupling reaction and a cysteinyl-desulfurization reaction, including recovered reactivity at red wavelengths where [Ru(bpy)3]2+ alone does not absorb." @default.
- W3213202893 created "2021-11-22" @default.
- W3213202893 creator A5011564912 @default.
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- W3213202893 date "2022-01-01" @default.
- W3213202893 modified "2023-10-12" @default.
- W3213202893 title "A biohybrid strategy for enabling photoredox catalysis with low-energy light" @default.
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- W3213202893 doi "https://doi.org/10.1016/j.chempr.2021.10.010" @default.
- W3213202893 hasPublicationYear "2022" @default.
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