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• W3213433441 abstract "The sequestration of organic luminescent molecules (OLMs) within cage-based metal-organic frameworks (MOFs) as a dispersion platform has been developed to impede aggregation-caused quenching (ACQ). The homogenous encapsulation of distinct luminescent guests of different sizes and emissive behaviors in the cage structure of a MOF resulted in high fluorescent quantum yields of 44.8% for DAPI@NKU-110 (DAPI = 4',6-diamidino-2-phenylindole), 65.4% for TPPA@NKU-110 (TPPA = tris(4-(pyridin-4- yl)phenyl)amine), 31.3% for R6G@NKU-110 (R6G = Rhodamine 6G), and 58.3% for PY@NKU-110 (PY = Pyronin Y), attributable to the confinement effect caused by the rigid cages of NKU-110. More significantly, a positive correlation of the encapsulated quantity of OLMs with their concentration in the in-situ solvothermal reaction was unveiled by spectral analysis and utilized to facilely fabricate a white-light-emitting crystal material TPPA+R6G@NKU-110. This material features a large crystal size on the millimeter-scale, broadband white emission, ideal CIE coordinates (0.33, 0.34), and a high quantum yield (49.1%) when excited at 365 nm. Moreover, such a strategy can be easily generalized to an abundance of other cage-based MOFs and a plentiful volume of OLMs for the future development of colorful, high performance luminescent materials. Appendix S1: Supporting Information Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article." @default.
• W3213433441 created "2021-11-22" @default.
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• W3213433441 date "2021-12-29" @default.
• W3213433441 modified "2023-09-27" @default.
• W3213433441 title "<scp>Crystalline‐State</scp> Solvent: <scp>Metal‐Organic</scp> Frameworks as a Platform for Intercepting <scp>Aggregation‐Caused</scp> Quenching" @default.
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• W3213433441 doi "https://doi.org/10.1002/cjoc.202100712" @default.
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