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- W3214054534 endingPage "133557" @default.
- W3214054534 startingPage "133557" @default.
- W3214054534 abstract "Sodium vanadium fluorophosphate has been extensively explored for the cathode of sodium ion batteries (SIBs), which is known for its high voltage platform, three-dimensional framework structure and minor volume deformation. However, low intrinsic electronic conductivity restricts its practical charge/discharge performances. Accelerating the electron/ion transport process of sodium vanadium fluorophosphate is the vital point to realize high performances of SIBs. Herein, a well-designed nitrogen doped three-dimensional (3D) nanosheet flower-like Na3V2(PO4)2F2.5O0.5 composite (N-NVPFO) is proposed by optimizing nanostructure plus heteroatom doping. The 3D flower-like structure of N-NVPFO provides a great deal of active sites and guarantees the structure stability. In addition, the N-doping in Na3V2(PO4)2F2.5O0.5 bulk phase could enhance the intrinsic electronic conductivity by narrowing the energy gap, which is confirmed through the density functional theoretical (DFT) calculation. The N-NVPFO electrode delivers excellent rate capability (84 mAh g−1 at 10C) and long cycling life (86% capacity retention up to 2000 cycles). Furthermore, the quasi-solid-state SIBs using NaTi2(PO4)3 anode also exhibits good electrochemical performances." @default.
- W3214054534 created "2021-11-22" @default.
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- W3214054534 date "2022-04-01" @default.
- W3214054534 modified "2023-10-17" @default.
- W3214054534 title "Optimizing quasi-solid-state sodium storage performance of Na3V2(PO4)2F2.5O0.5 cathode by structural design plus nitrogen doping" @default.
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- W3214054534 doi "https://doi.org/10.1016/j.cej.2021.133557" @default.
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