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• W3214575450 endingPage "20130" @default.
• W3214575450 startingPage "20117" @default.
• W3214575450 abstract "In this study, we propose that the multistep, tandem catalytic fast hydropyrolysis (CFHP) and hydrotreatment reactions of biomass to produce gasoline and diesel grade biofuels can be conducted in a single step process using a composite of Ni-ZSM-5 microcrystals encapsulated in spherical particles of Ni-MCM-41 (Ni-ZSM-5/Ni-MCM-41). The composite has been successfully prepared via a one-step aerosol method and characterized by N2 adsorption–desorption, X-ray diffraction, scanning electron microscope (SEM), transmission electron microscope (TEM), pyridine adsorption, inductively coupled plasma-optical emission spectrometry (ICP-OES), and H2 chemisorption. The composite has been tested for one-stage CFHP and hydrotreatment of Miscanthus × giganteus at 600 and 500 °C. The product yields and distribution derived from the one-stage CFHP and hydrotreatment of Miscanthus × giganteus using the Ni-ZSM-5/Ni-MCM-41 composite were compared to those of a typical two-stage process, with Ni-ZSM-5 in the first stage (CFHP) and Ni-MCM-41 in the second stage (hydrotreatment). Additional experiments were carried out using Ni-ZSM-5, Ni-ZSM-5/MCM-41, and ZSM-5/Ni-MCM-41 composites, as well as physical mixtures of Ni-ZSM-5 and Ni-MCM-41 to obtain further insights into the role of each part of the composites to the product yields and distribution derived from the one-stage CFHP and hydrotreatment reaction. The comparison of results showed that the Ni-ZSM-5/Ni-MCM-41 composite enhanced the production of alkanes and methane without sacrificing the yield to monoaromatic hydrocarbons. Therefore, this study proves that such a unique composite can complete the two-step tandem reactions in one single step, leading to a self-sustainable and intensified process." @default.
• W3214575450 created "2021-11-22" @default.
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• W3214575450 date "2021-11-12" @default.
• W3214575450 modified "2023-09-26" @default.
• W3214575450 title "One-Step Hydropyrolysis and Hydrotreating Tandem Reactions of <i>Miscanthus × giganteus</i> Using Ni Impregnated ZSM-5/MCM-41 Composites" @default.
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• W3214575450 doi "https://doi.org/10.1021/acs.energyfuels.1c02453" @default.
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