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- W3214861622 abstract "We reveal the effects of ions on the oil–water wettability of rock surfaces, which originally adsorb polar molecules via ion-bridging interactions. The ion-induced oil-water wettability alteration is instead revealed by using molecular dynamics simulations, owing to the difficult in the realization of ion-bridging interactions in a hydrated water film in experiments. The results show that the spontaneous displacement of Ca2+ ions in water film by Na+ ions in bulk water phase can weaken the ion-bridging effect and accordingly the rock surface becomes more water-wet. A maximum decrease of approximately 20° in the water contact angle is observed in a period of 30 ns at 0.5 mol/L of Na+ ions. The displacement is guaranteed because smaller Na+ ions can easily embed into silica structure and subsequently weaken the electronegativity of rock surfaces. This study gives a molecular insight of the mechanism of wettability alteration on rock surfaces under ion-bridging interactions." @default.
- W3214861622 created "2021-12-06" @default.
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- W3214861622 date "2022-04-01" @default.
- W3214861622 modified "2023-10-14" @default.
- W3214861622 title "Ion-induced oil–water wettability alteration of rock surfaces. Part III: Ion-bridging interactions between oil and solid" @default.
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- W3214861622 doi "https://doi.org/10.1016/j.ces.2021.117275" @default.
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