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• W3214944038 abstract "Abstract We present a novel approach to transient Raman spectroscopy, which combines stochastic probe pulses and a covariance-based detection to measure stimulated Raman signals in alpha-quartz. A coherent broadband pump is used to simultaneously impulsively excite a range of different phonon modes, and the phase, amplitude, and energy of each mode are independently recovered as a function of the pump–probe delay by a noisy-probe and covariance-based analysis. Our experimental results and the associated theoretical description demonstrate the feasibility of 2D-Raman experiments based on the stochastic-probe schemes, with new capabilities not available in equivalent mean-value-based 2D-Raman techniques. This work unlocks the gate for nonlinear spectroscopies to capitalize on the information hidden within the noise and overlooked by a mean-value analysis." @default.
• W3214944038 created "2021-12-06" @default.
• W3214944038 creator A5053942567 @default.
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• W3214944038 date "2022-03-01" @default.
• W3214944038 modified "2023-10-14" @default.
• W3214944038 title "Transient measurement of phononic states with covariance-based stochastic spectroscopy" @default.
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• W3214944038 doi "https://doi.org/10.1038/s41377-022-00727-6" @default.
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