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- W3215394543 abstract "Abstract Chemo-switchable catalytic [2+2+2] cycloaddition of alkenes with formaldimines is reported. Bis(tosylamido)methane (BTM) and 1,2-ditosyl-1,2-diazetidine (DTD), two bench-stable precursors for highly reactive tosylformaldimine, have been identified to be effective. BTM worked as a selective releaser of the formaldimine for catalytic [2+2+2] reactions toward hexahydropyrimidine products via a presumable ‘imine–alkene–imine’ addition. A unique catalytic retro-[2+2] reaction of DTD was used and has enabled a proposed ‘imine–alkene–alkene’ pathway with high chemoselectivity for the synthesis of 2,4-diarylpiperidine derivatives. The two alternative processes are catalyzed by the simple and environmentally benign catalysts InCl3 and FeBr2, respectively." @default.
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- W3215394543 date "2021-12-01" @default.
- W3215394543 modified "2023-10-16" @default.
- W3215394543 title "Catalytic Amidomethylative [2+2+2] Cycloaddition of Formaldimine and Styrenes toward N-Heterocycles" @default.
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- W3215394543 doi "https://doi.org/10.1055/a-1710-7256" @default.
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