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- W3215671942 abstract "The active sites of monodisperse transition metal Ni-clusters were anchored on carbon nitride (CN) by an in situ photoreduction deposition method to promote the efficient separation of photogenerated charges and achieve high-efficiency photocatalytic activity for hydrogen evolution. The Ni-cluster/CN exhibited a photocatalytic hydrogen production rate of 16.5 mmol·h–1·g–1 and a total turnover frequency (TOF (H2)) value of 461.14 h–1. X-ray absorption spectroscopy based on synchrotron radiation indicated that CN had two reaction centers to form stable interface interactions with monodispersed Ni-clusters, in which carbon can act as an electron acceptor, while nitrogen can act as an electron donor. Meanwhile, the hybrid electronic structure of the Ni-cluster/CN system was constructed, which was favorable for photocatalytic activity for hydrogen production. An in-depth understanding of the interfacial interaction between CN and Ni-clusters will have important reference significance on the mechanistic study of development based on the cocatalyst." @default.
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- W3215671942 date "2022-02-01" @default.
- W3215671942 modified "2023-10-18" @default.
- W3215671942 title "Monodisperse Ni-clusters anchored on carbon nitride for efficient photocatalytic hydrogen evolution" @default.
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- W3215671942 doi "https://doi.org/10.1016/s1872-2067(21)63865-2" @default.
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