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- W3216217576 abstract "High-voltage and low-cost manganese-based P2-type oxides show real promise as promising cathode for sodium-ion batteries (SIBs). But the P2 - O2 phase transformation and Na+/vacancy ordering results in the inferior structural stability and Na+ diffusion coefficient, which further leads to rapid decay of capacity and poor rate capability. Herein, in consideration of the synergetic effects of dual cationic doping, electrochemically inactive Li+ and active Co3+ codoping are proposed to solve the above issues. The novel two-step doping strategy, Co doping during synthesis of precursors via coprecipitation reaction followed by Li doping during solid-state reaction, are rationally developed. As anticipated, the Li/Co codoped P2-type oxide exhibits the absence of P2 - O2 phase transformation and Na+/vacancy disordering, which gives rise to an outstanding cycling stability (86.7% capacity retention within 100 cycles at 0.1C) and high-rate capability (reversible capacity of 109 mAh g-1 even at 10C). In addition, the full-cells composed of the codoped P2-type positive and hard carbon negative show high energy-density, good lifespan and high-rate property. This proposed cationic codoping provides an effective and scalable tactics for modulating the structural properties of high-voltage P2-type cathodes for advanced SIBs." @default.
- W3216217576 created "2021-12-06" @default.
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- W3216217576 date "2022-04-01" @default.
- W3216217576 modified "2023-10-17" @default.
- W3216217576 title "Suppressing the P2 − O2 phase transformation and Na+/vacancy ordering of high-voltage manganese-based P2-type cathode by cationic codoping" @default.
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- W3216217576 doi "https://doi.org/10.1016/j.jcis.2021.11.171" @default.
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