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- W3216285414 abstract "The tandem reactions of CO2-assisted oxidative dehydrogenation and aromatization (CO2-ODA) of ethane were investigated over ZSM-5 modified with zinc (Zn) and phosphorus (P) by experimental studies and DFT calculations. The nature of active Zn species and their interaction with P were elucidated for understanding Zn/P-ZSM-5 catalyzed CO2-ODA reaction of ethane. Compared to the direct dehydrogenation and aromatization (DDA) reaction, the Zn/P-ZSM-5 catalyst possessed higher ethane conversion, enhanced aromatics yield, and better stability in the CO2-ODA reaction. The presence of CO2 reduced the carbon deposition, stabilized the Zn species, and thereby facilitated the generation of more liquid aromatics in CO2-assisted ethane aromatization. In situ characterization and DFT calculations provided insight into the mechanisms of CO2-ODA over the Zn/P-ZSM-5 catalyst." @default.
- W3216285414 created "2021-12-06" @default.
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- W3216285414 date "2022-05-01" @default.
- W3216285414 modified "2023-10-10" @default.
- W3216285414 title "CO2-assisted ethane aromatization over zinc and phosphorous modified ZSM-5 catalysts" @default.
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- W3216285414 doi "https://doi.org/10.1016/j.apcatb.2021.120956" @default.
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