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- W3216495261 abstract "Rotationally-resolved infrared spectra of N 2 O–Ar and N 2 O–Kr are studied in the region of the N 2 O ν 1 vibration (≈2224 cm −1 ) using a tunable Quantum Cascade laser source to probe a pulsed supersonic jet. The N 2 O–Kr ν 1 fundamental band is re-analyzed, together with previous ν 3 band data, using a unified scheme to fit the (small) observed Kr isotope splittings. This scheme is then transferred to analyze the bending combination band of N 2 O–Kr near 2257 cm −1 where isotope effects are much larger due to stretch-bend interactions. As a result, N 2 O–Kr intermolecular bend (33.29 cm −1 ) and stretch (34.48 cm −1 ) frequencies are directly determined for the first time. Weak spectra are detected for both N 2 O–Ar and –Kr corresponding to the (ν 1 , ν 2 l 2 , ν 3 ) = (11 1 0) ← (01 1 0) hot band of N 2 O. Their analysis yields the magnitude of the splitting of the N 2 O ν 2 bending mode into in-plane and out-of-plane components. These splittings are found to be significantly smaller than those observed in the analogous CO 2 -containing dimers." @default.
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- W3216495261 date "2022-01-01" @default.
- W3216495261 modified "2023-09-24" @default.
- W3216495261 title "N2O–Ar and N2O–Kr: intermolecular vibrations of N2O–Kr and symmetry breaking of the N2O bending mode in the presence of a rare gas" @default.
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- W3216495261 doi "https://doi.org/10.1016/j.jms.2021.111551" @default.
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