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• W3216605516 endingPage "569" @default.
• W3216605516 startingPage "562" @default.
• W3216605516 abstract "A series of trinuclear complexes, [MnII2YIII(L)2(HL)2(NO3)3][YIII(NO3)5]·7H2O (1'), [MnII2GdIII(HL)4(NO3)4]2[MnII2GdIII(L)(HL)3(NO3)4][GdIII(NO3)5]4·2(o-Xy)·12H2O (2') and [MnII3(L)(HL)2(NO3)4](NO3)·1.25(p-Xy) (3'), were synthesized using a β-diketone ligand HL (HL = 1,3-bis(pyridin-2-yl)propane-1,3-dione). X-ray structural analyses revealed that each complex has a trinuclear core with an Mn(II)-M-Mn(II) arrangement (M = YIII (1), GdIII (2), and MnII (3)). In 1' with a diamagnetic Y(III) ion, negligible antiferromagnetic interactions between terminal Mn(II) ions are operative. On the other hand, 2' shows ferromagnetic interactions between Mn(II) and Gd(III) ions, affording a spin ground state of ST = 17/2. The homometallic Mn(II)3 complex of 3' has an ST = 5/2 spin ground state resulting from the antiferromagnetic interactions between neighboring Mn(II) ions. The maximum magnetic entropy change (-ΔSm) of 1'-3' was estimated to be 12.3, 24.8, and 8.0 J kg-1 K-1, respectively." @default.
• W3216605516 created "2021-12-06" @default.
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• W3216605516 date "2022-01-01" @default.
• W3216605516 modified "2023-10-17" @default.
• W3216605516 title "Syntheses, structures, and magnetic properties of a series of Mn–M–Mn trinuclear complexes with different spin configurations" @default.
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• W3216605516 doi "https://doi.org/10.1039/d1dt03030b" @default.
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