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- W3216977201 abstract "Transition metal-catalyzed cycloaddition has been established as a powerful tool for heterocycle synthesis. Despite impressive advances, the exploitation of new catalysis strategies and systems is still highly significant to enrich the heterocycle family. Herein, we disclosed a cooperative catalysis system merging an achiral Pd catalyst and a chiral Co catalyst for the asymmetric [4+2] cycloaddition between vinyl benzoxazinones and N-acylpyrazoles. Chiral tetrahydroquinolines bearing two contiguous, unusual cis-configured stereocenters were produced in high yields and enantio- and diastereoselectivities. The pyrazole directing group can be easily converted into many other functional groups, thus demonstrating the flexibility of the present methodology." @default.
- W3216977201 created "2021-12-06" @default.
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- W3216977201 date "2021-01-01" @default.
- W3216977201 modified "2023-10-17" @default.
- W3216977201 title "A cooperative Pd/Co catalysis system for the asymmetric (4+2) cycloaddition of vinyl benzoxazinones with <i>N</i>-acylpyrazoles" @default.
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- W3216977201 doi "https://doi.org/10.1039/d1cc05952a" @default.
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