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• W3217050281 startingPage "645" @default.
• W3217050281 abstract "Synergistic doping of the metastable Gd3Al5O12:Ce garnet with a Ca2+/Hf4+ pair and Sc3+ to form Gd2.97-xCaxHfxScyAl3O12:0.03Ce (x = 0.5-2.0, y = 0.0-1.5, x + y = 2.0) solid solution was conducted for the structural stabilization and photoluminescence manipulation. The site selection of Ca2+/Hf4+/Sc3+ dopants and the effects of doping on the crystal structure, local coordination, band structure and Ce3+ luminescence were revealed in detail with the results of XRD, Rietveld refinement, TEM, and UV-Vis/photoluminescence spectroscopy. A decrease in Ca2+/Hf4+ and an increase in the Sc3+ content were observed to shrink the lattice, widen the bandgap of the garnet host, red-shift the excitation/emission wavelength, broaden the emission band and shorten the fluorescence lifetime of Ce3+. The spectral changes were rationalized by considering the local coordination and crystal field splitting of the Ce3+ 5d energy level. Application of typical Gd0.97Ca2Hf2Al3O12:0.03Ce (x = 2.0, y = 0) cyan and Gd2.47Ca0.5Hf0.5Sc1.5Al3O12:0.03Ce (x = 0.5, y = 1.5) greenish-yellow phosphors in w-WLED lighting produced low correlated color temperatures of ∼3842 and 3514 K, high color rendering indices of ∼88 and 93 and favorable luminous efficacies of ∼32.9 and 14.7 lm/W under the excitation of 395 nm n-UV and 450 nm blue LED chips, respectively." @default.
• W3217050281 created "2021-12-06" @default.
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• W3217050281 date "2022-01-01" @default.
• W3217050281 modified "2023-10-15" @default.
• W3217050281 title "Site-selective and cooperative doping of Gd₃Al₅O₁₂:Ce garnets for structural stabilization and warm WLED lighting of low CCT and high CRI" @default.
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• W3217050281 doi "https://doi.org/10.1039/d1dt03599a" @default.
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• W3217050281 hasPublicationYear "2022" @default.
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