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- W3217424242 abstract "Amorphous, porous materials represent by far the largest proportion of natural and men-made materials. Their pore networks consists of a wide range of pore sizes, including meso- and macropores. Within such a pore network, material moisture plays a crucial role in almost all transport processes. In the hygroscopic range, the pores are partially saturated and liquid water is only located at the pore fringe due to physisorption. Therefore, material parameters such as porosity or median pore diameter are inadequate to predict material moisture and moisture transport. To quantify the spatial distribution of material moisture, Hillerborg's adsorption theory is used to predict the water layer thickness for different pore geometries. This is done for all pore sizes, including those in the lower nanometre range. Based on this approach, it is shown that the material moisture is almost completely located in mesopores, although the pore network is highly dominated by macropores. Thus, mesopores are mainly responsible for the moisture storage capacity, while macropores determine the moisture transport capacity, of an amorphous material. Finally, an electrical analogical circuit is used as a model to predict the diffusion coefficient based on the pore-size distribution, including physisorption." @default.
- W3217424242 created "2021-12-06" @default.
- W3217424242 creator A5007261490 @default.
- W3217424242 creator A5010089707 @default.
- W3217424242 creator A5016352216 @default.
- W3217424242 date "2021-11-27" @default.
- W3217424242 modified "2023-09-25" @default.
- W3217424242 title "About the Dominance of Mesopores in Physisorption in Amorphous Materials" @default.
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- W3217424242 doi "https://doi.org/10.3390/molecules26237190" @default.
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- W3217424242 hasPublicationYear "2021" @default.
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