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• W3217496795 abstract "The electrochemical CO2 reduction reaction (CO2 RR) over Cu-based catalysts shows great potential for converting CO2 into multicarbon (C2+ ) fuels and chemicals. Herein, we introduce an A2 M2 O7 structure into a Cu-based catalyst through a solid-state reaction synthesis method. The Cu2 P2 O7 catalyst is electrochemically reduced to metallic Cu with a significant structure evolution from grain aggregates to highly porous structure under CO2 RR conditions. The reconstructed Cu2 P2 O7 catalyst achieves a Faradaic efficiency of 73.6 % for C2+ products at an applied current density of 350 mA cm-2 , remarkably higher than the CuO counterparts. The reconstructed Cu2 P2 O7 catalyst has a high electrochemically active surface area, abundant defects, and low-coordinated sites. In situ Raman spectroscopy and density functional theory calculations reveal that CO adsorption with bridge and atop configurations is largely improved on Cu with defects and low-coordinated sites, which decreased the energy barrier of the C-C coupling reaction for C2+ products." @default.
• W3217496795 created "2021-12-06" @default.
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• W3217496795 date "2021-12-10" @default.
• W3217496795 modified "2023-10-16" @default.
• W3217496795 title "A Reconstructed Cu₂P₂O₇ Catalyst for Selective CO₂ Electroreduction to Multicarbon Products" @default.
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• W3217496795 doi "https://doi.org/10.1002/anie.202114238" @default.
• W3217496795 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34859554" @default.
• W3217496795 hasPublicationYear "2021" @default.
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