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- W3217770507 abstract "Abstract A 1 : 2 mixture of Zn‐ meso ‐tetrakis(4‐dodecyl‐3,5‐dihydroxyphenyl)porphyrin ( 1‐Zn ) and tetrakis(4‐pyridylethynyl)cavitand ( 2 ) in C 6 D 6 self‐assembles quantitatively into the doubly cavitand‐capped Zn‐porphyrin capsule 2 ⋅ 1‐Zn ⋅ 2 with two cavities divided by the porphyrin ring via eight ArOH⋅⋅⋅Npy hydrogen bonds. Simultaneous encapsulation of 1‐acetoxy‐3,5‐dimethoxybenzene ( G ) and 4‐(4‐methylphenyl)pyridine ( L2 ) in 2 ⋅ 1‐Zn ⋅ 2 preferentially occurs to form G / L2 @( 2 ⋅ 1‐Zn ⋅ 2 ). A 1 : 1 mixture of 1‐Zn and 2 in the presence of G and L2 self‐assembles into the G ‐encapsulating half‐capsule G @( 2 ⋅ 1‐Zn ) ⋅ L2 with coordination of L2 at the outer side of 2 ⋅ 1‐Zn . A 2 : 2 : 1 mixture of 1‐Zn , 2 , and 1,4‐diazabicyclo[2.2.2]octane ( L3 ) in the presence of G self‐assembles preferentially into the G ‐encapsulating doubly cavitand‐capped double‐decker Zn‐porphyrin capsule G / G @( 2 ⋅ 1‐Zn ⋅ L3 ⋅ 1‐Zn ⋅ 2 ) with coordination of L3 between two hydrogen‐bonded 1‐Zn subunits. Thus, selective formation of these cavitand–porphyrin capsules can be controlled by the stoichiometry of 1‐Zn and 2 as well as the character of N‐ligands." @default.
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- W3217770507 date "2021-12-16" @default.
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- W3217770507 title "Doubly Cavitand‐Capped Zn‐Porphyrin Capsule with Simultaneous Encapsulation of Guest and Ligand, and Its Application to Doubly Cavitand‐Capped Double‐Decker Zn‐Porphyrin Capsule" @default.
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- W3217770507 doi "https://doi.org/10.1002/ajoc.202100646" @default.
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