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- W3217809384 abstract "For rechargeable lithium–metal batteries (RLBs), gel polymer electrolytes (GPEs) are a very competitive and pragmatic option because the special composite structure could restrain the uncontrolled lithium dendrite in a liquid electrolyte and avoid the poor interface contact for a solid-state electrolyte. However, the difficulty lies in finding a delicate balance between ion transport and interface stability. Herein, a heterostructured GPE, in which a metal–organic framework layer and an ultrathin Al2O3 deposition are coated on the same side of a polymer matrix, is fabricated to homogenize lithium ion transport and stabilize the lithium anode interface. With the heterostructured GPE, the Li+ transference number is improved to 0.74, and the lithium metal electrode displays an enhanced cycle stability over 1000 h. Moreover, Li-rich Mn-based layered oxides, the high-capacity cathode material, are matched for the first time with a lithium–metal anode to assemble a quasi-solid-state RLB, which delivers an initial discharge capacity of 257.5 mAh g–1 with a long-cycle capacity retention of 84.6% after 500 cycles at a rate of 0.2C." @default.
- W3217809384 created "2021-12-06" @default.
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- W3217809384 date "2021-11-29" @default.
- W3217809384 modified "2023-10-16" @default.
- W3217809384 title "Heterostructured Gel Polymer Electrolyte Enabling Long-Cycle Quasi-Solid-State Lithium Metal Batteries" @default.
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- W3217809384 doi "https://doi.org/10.1021/acsenergylett.1c02233" @default.
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