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- W34099076 abstract "There is a large body of theoretical work on the transition from the molecular to the solid state in metallic clusters. Theoretical studies of the electronic and magnetic properties of metallic clusters indicate that the appearance of solid state behavior, such as the emergence of a conduction band and collective magnetic phenomena, occur at the vicinity of N∼10, where N is the number of atoms in the cluster. This chapter presents experimental work on the transition region between molecular and bulk magnetic behavior. It discusses magnetic properties of supramolecular ferric oxo/hydroxo particles, that is, large molecular complexes that contain an increasing number of super-exchange-coupled iron (III) ions obtained through controlled chemical synthesis. The chapter presents experimental criteria that establish the onset of incipient solid-state magnetic correlation effects. These chemical structures are beyond the molecular realm but convergence to the bulk has not yet been attained. Fundamental new properties associated with quantum size effects are expected. Unraveling the physical properties of matter at the molecular/solid state boundary can, in principle, open up new areas of applications and theoretical approaches to the electronic and magnetic properties of materials." @default.
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- W34099076 date "1993-01-01" @default.
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- W34099076 title "Supramolecular Particles: The Transition from the Molecular to the Solid State" @default.
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- W34099076 doi "https://doi.org/10.1016/b978-0-444-89022-1.50024-9" @default.
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