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- W346983043 abstract "Non-dipole electronic transitions in 7-10 eV have been observed in a series of chlorofluoromethanes, CF{sub 4-n}Cl{sub n} (n=1-3), using angle-resolved electron energy loss spectroscopy at 2.5 keV impact energy. The generalized oscillator strengths of these low-lying non-Rydberg transitions have been determined and found to have a shape characteristic of a quadrupole-allowed transition. Ab-initio single-excitation CI calculations show that some of these quadrupole states correspond to predissociation channels due to the breakage of the C-Cl bond. Some plausible spectral assignments and related processes of these non-dipole transitions will be discussed. Furthermore, the GOS measurement of Cl 2p and Cls transitions also gives evidence for the presence of non-dipole processes in the inner shells." @default.
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- W346983043 date "1993-05-01" @default.
- W346983043 modified "2023-09-27" @default.
- W346983043 title "Observation of new multipole electronic transitions in chlorofluoromethanes: Generalized oscillator strength measurements by angle-resolved electron energy loss spectroscopy" @default.
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