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- W36115459 abstract "Using in situ Raman spectroscopy and resistance measurements we demonstrate the existence of a whole family of azafulleride ${mathrm{Rb}}_{x}{mathrm{C}}_{59}mathrm{N}$ phases. Six phases with $x=1,2,3,4,5,6$ were identified from a detailed spectroscopic study of the intercalation physics and chemistry. Intriguingly, the most stable phases were observed for ${mathrm{RbC}}_{59}mathrm{N},$ ${mathrm{Rb}}_{2}{mathrm{C}}_{59}mathrm{N},$ and ${mathrm{Rb}}_{4}{mathrm{C}}_{59}mathrm{N}$ whereas minimum resistance was observed for ${mathrm{Rb}}_{3}{mathrm{C}}_{59}mathrm{N}.$ This supports a strong localization of the extra charge density introduced by the nitrogen substitution for all stable phases. These findings together with the observation that the dimer dissociates before ${mathrm{RbC}}_{59}mathrm{N}$ is formed allowed us to get insight into the effects of cage distortion and chemical doping as well as into the electronic properties of fullerene intercalation compounds." @default.
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- W36115459 date "2001-03-21" @default.
- W36115459 modified "2023-09-23" @default.
- W36115459 title "Phases for the azafulleridesRbxC59N" @default.
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- W36115459 doi "https://doi.org/10.1103/physrevb.63.140301" @default.
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