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- W36388762 abstract "Synthesis gas can be produced by the autothermal direct oxidation of methane over rhodium coated monoliths at contact times on the order of several milliseconds. Modeling these reactors is useful both to better understand the system as well as to predict operation in regimes where experiments are either difficult or dangerous. These systems are difficult to model because the gradients are very large, parameters are strong functions of temperature and concentration, and the processes are very sensitive to catalyst geometry. We have simulated these processes using both a plug flow model to investigate the detailed gas phase and surface chemistry within the monolith as well as a 2-dimensional model to investigate the role of temperature and composition dependent transport with spatial gradients in temperature, concentration, and velocity." @default.
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- W36388762 date "1998-01-01" @default.
- W36388762 modified "2023-10-18" @default.
- W36388762 title "Modeling the Partial Oxidation of Methane to Syngas at Millisecond Contact Times" @default.
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- W36388762 doi "https://doi.org/10.1016/s0167-2991(98)80511-9" @default.
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