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- W373321901 abstract "Coherent wavepacket motions of 5,12-bis(phenylethynyl)-naphthacene (BPEN) in an inert solvent, 1-chloronaphthalene (1-CN), and in an electron donating solvent, N,N-dimethylaniline (DMA) were compared by femtosecond white-light supercontinuum transient absorption (WC-TA) spectroscopy. In the inert solvent, 1-CN, both the intensity and the wavelength of the stimulated emission (SE) was modulated by the wavepacket motion, i.e., the maximum of the SE spectrum exhibited a repetitive movement between longer and shorter wavelengths (frequency-modulation) and the SE intensity was stronger at shorter wavelengths (amplitude-modulation). While in the electron donating solvent, DMA, the intensity was quickly diminished and only the frequency-modulation remained. The ultrafast electron transfer (ET) occurring in a few picosecond range rapidly diminishes the population in the vicinity of the Franck–Condon region and the wavepacket motion was no longer capable of recovering the SE intensity." @default.
- W373321901 created "2016-06-24" @default.
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- W373321901 date "2015-12-01" @default.
- W373321901 modified "2023-10-16" @default.
- W373321901 title "Femtosecond coherent wavepacket motion in an ultrafast electron transfer system composed of naphthacene derivative in an electron donating solvent" @default.
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- W373321901 doi "https://doi.org/10.1016/j.jphotochem.2015.05.014" @default.
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