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- W397719907 abstract "The superionic transitions of protonated K3H(SO4)2 and deuterated K3D(SO4)2 insulators are investigated using Raman scattering and differential scanning calorimetry (DSC) measurements. DSC indicates that the superionic transition temperature of K3D(SO4)2 is approximately 9 K lower than that of K3H(SO4)2. This confirms the negative isotope effect on the superionic transition temperature of this compound and suggests that the bonding strength of D bonds is lower than that of H bonds. Raman scatterings from K3H(SO4)2 and K3D(SO4)2 show that the ν1-normal vibration mode of the SO4 tetrahedra consists of two rather than one band, despite the symmetry of the vibration mode. The oscillation frequency of the ν1-mode for SO4 tetrahedra in K3D(SO4)2 is higher than that for K3H(SO4)2, which is thought to be closely related to the negative isotope effect on the transition temperature." @default.
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- W397719907 date "2013-10-15" @default.
- W397719907 modified "2023-10-14" @default.
- W397719907 title "Negative Isotope Effect on the Superionic Transition Point and the Behavior of the SO4ν1-Internal Modes in K3H(SO4)2and K3D(SO4)2" @default.
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- W397719907 doi "https://doi.org/10.7566/jpsj.82.104601" @default.
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