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- W40392378 abstract "Static light-scattering measurements on aqueous solutions of charged polystyrenesulfonate (PSS) with five molecular weights between 1100 000 g/mol and 1 132 000 g/mol are presented. All experiments were performed in the dilute/semidilute regime at minimum ionic strengths (≈ 10−6 M) in order to maximize the electrostatic interaction between monomers of different polymers or monomers belonging to the same polymer. A single broad peak in the scattered intensity was always found. The scattering vectors of these peaks increase with increasing concentrations c and scale either with c 1/3 or with c 1/2, depending on concentration: Below about 20 c*{1c*:=1 particle/(contour lengths l c )3}, we found the c 1/3 dependence of the scattering vector; above 20 c*, the c 1/2 law is valid. A very similar behavior has been observed for rigid rods [1]. Furthermore, our results are compared with previous light-[2,3], small-angle neutron-[4] and small-angle x-ray [5]-scattering investigations. Nearly all of these studies confirm the validity of the c 1/3- and c 1/2-law, respectively. It is claimed that these laws can be explained by a flexibility of more or less strongly elongated PSS-rods which decreases with increasing molecular weight. Theories calculating the persistence lengths of charged linear polymers [6], and measurements of the electric birefringence being performed at present confirm our findings." @default.
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- W40392378 date "2007-12-10" @default.
- W40392378 modified "2023-09-26" @default.
- W40392378 title "Static light scattering by aqueous, salt-free solutions of charged polystyrenesulfonate at different molecular weights" @default.
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- W40392378 doi "https://doi.org/10.1007/bfb0115132" @default.
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