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• W4200011723 endingPage "106871" @default.
• W4200011723 startingPage "106871" @default.
• W4200011723 abstract "Unstable solid-electrolyte interphase (SEI) layer, accompanied with detrimental Li dendrite growth, is the major challenge for realizing viable Li metal batteries. Herein, we report a self-healing and single-ion conductive artificial SEI (SS-ASEI) layer to stabilize Li metal anode, suppress the Li dendrite growth and promote the Li plating/stripping kinetics. The polymeric SS-ASEI layer is optimized to be dynamically cross-linked poly(dimethylsiloxane) filled with 7 wt% SiO 2 nanoparticles. The modified Li symmetric cell achieves extremely stable plating/stripping cycling for 1340 h at 0.5 mA cm −2 and 1.0 mAh cm −2 cutting-off capacity. Superior rate capability and cycling stability of the modified anode are also demonstrated in cells with commercial NCM811 (LiNi 0.8 Co 0.1 Mn 0.1 O 2 ) cathode. The self-healing ability, elastic deformation capability, selectively high Li-ion conductivity and low liquid electrolyte swelling rate of our SS-ASEI layer synergistically account for the superior performances of modified Li electrode over the bare Li electrode. A polymeric artificial solid-electrolyte interphase layer , with elastic deformation ability, highly selective Li-ion conductivity and quick self-healing capability, is designed for stabilizing dendrite-free lithium-metal anodes. • A self-healing and single-ion-conductive artificial SEI layer is proposed to stabilize Li-metal anodes. • The ion-conducting performances of the polymeric SEI layer is optimized with inorganic SiO 2 nanoparticles fillers. • Stable and longlife Li plating/stripping is achieved with the aid of this artificial SEI layer. • The superior rate capability and cycling stability is achieved for high-voltage Li-metal battery." @default.
• W4200011723 created "2021-12-31" @default.
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• W4200011723 date "2022-03-01" @default.
• W4200011723 modified "2023-10-17" @default.
• W4200011723 title "Self-healing single-ion-conductive artificial polymeric solid electrolyte interphases for stable lithium metal anodes" @default.
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• W4200011723 doi "https://doi.org/10.1016/j.nanoen.2021.106871" @default.
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