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- W4200014166 abstract "As a model molecule of actinide chemistry, UO molecule plays an important role in understanding the electronic structure and chemical bonding of actinide-containing species. We report a study of the laser-induced fluorescence spectra of the U 16 O and U 18 O using two-dimensional spectroscopy. Several rotationally resolved excitation spectra were investigated. Accurate molecular rotational constants and equilibrium internuclear distances were reported. Low-lying electronic states information was extracted from high resolution dispersed fluorescence spectra and analyzed by the ligand field theory model. The configuration of the ground state was determined as U 2+ (5f 3 7s)O 2− . The branching ratios, and the vibrational harmonic and anharmonic parameters were also obtained. Radiative lifetimes were determined by recording the time-resolved fluorescence spectroscopy. Transition dipole moments were calculated using the branching ratios and the radiative lifetimes. These findings were elucidated by using quantum-chemical calculations, and the chemical bonding was also analyzed. The findings presented in this work will enrich our understanding of actinide-containing molecules." @default.
- W4200014166 created "2021-12-31" @default.
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- W4200014166 date "2022-05-01" @default.
- W4200014166 modified "2023-09-27" @default.
- W4200014166 title "Laser-induced fluorescence experimental spectroscopy and theoretical calculations of uranium monoxide" @default.
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- W4200014166 doi "https://doi.org/10.1088/1674-1056/ac43a4" @default.
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