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• W4200047375 abstract "Controlling magnetic anisotropy is a key requirement for the fundamental understanding of molecular magnetism and is a prerequisite for numerous applications in magnetic storage, spintronics, and all-spin logic devices. In order to address the question of molecular magnetic anisotropy experimentally, we have synthesized single crystals of a molecular spin system containing four antiferromagnetically coupled s=5/2 manganese(II) ions. Using low-temperature cantilever magnetometry, we demonstrate the selective population of the S=0,1,...,10 spin states upon application of magnetic fields up to 33 T and map the magnetic anisotropy of each of these states. We observe a strong dependence of the shape and size of the magnetic anisotropy on the populated spin states, and, in particular, reveal an anisotropy reversal upon going from the lowest to the highest spin state.Received 19 August 2021Accepted 27 October 2021DOI:https://doi.org/10.1103/PhysRevResearch.3.L042042Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI.Published by the American Physical SocietyPhysics Subject Headings (PhySH)Research AreasMagnetic anisotropyMagnetic interactionsPhysical SystemsAntiferromagnetsMolecular magnetsTechniquesMagnetismMagnetization measurementsCondensed Matter, Materials & Applied Physics" @default.
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• W4200047375 date "2021-12-16" @default.
• W4200047375 modified "2023-10-14" @default.
• W4200047375 title "Magnetic anisotropy of individually addressed spin states" @default.
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• W4200047375 doi "https://doi.org/10.1103/physrevresearch.3.l042042" @default.
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