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• W4200150411 abstract "A facile one-step sonochemical activation method is utilized to fabricate biomass-derived 3D porous hard carbon (PHC-1) with tuned-surface and is compared with the conventional two-step activation method. As raw biomass offers good KOH impregnation, ultrasonication power diffuses both K+ and OH- ions deep into its interior, creating various nanopores and attaching copious functional groups. In contrast, conventional activation lacks these features under the same carbonization/activation parameters. The high porosity (1599 m2/g), rich functional groups (O = 8.10%, N = 0.95%), and well-connected nanoporous network resulting from sonochemical activation, remarkably increased specific capacity, surface wettability, and electrode stability, consequently improved electrochemical performance. Benefiting from its suitable microstructure, PHC-1 possesses superior specific capacity (330 mAh/g at 20 mA/g), good capacity retention (89.5%), and excellent structural stability over 500 sodiation/desodiation cycles at high current density (1000 mA/g). Apart from modus operandi comparison, the two activation methods also provide mechanistic insights as the low-voltage plateau region and graphitic layers decrease simultaneously. This work suggests a scalable and economical approach for synthesizing large-scale activated porous carbons that are used in various applications, be it energy storage, water purification, or gas storage, to name a few." @default.
• W4200150411 created "2021-12-31" @default.
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• W4200150411 date "2022-04-01" @default.
• W4200150411 modified "2023-10-15" @default.
• W4200150411 title "One-step sonochemical fabrication of biomass-derived porous hard carbons; towards tuned-surface anodes of sodium-ion batteries" @default.
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• W4200150411 doi "https://doi.org/10.1016/j.jcis.2021.12.104" @default.
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