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• W4200191539 startingPage "11360" @default.
• W4200191539 abstract "The complex modulus and the strain-optical coefficient for two samples of poly-γ-benzyl-l-glutamate in m-cresol solution were measured over a wide concentration regime covering from a dilute to tightly entangled region. The obtained experimental data in the dilute region were compared with the theory by Morse and coworkers for dilute solutions, which predicts three relaxation modes, tension, curvature, and orientation. We found that the theory well described the complex modulus of dilute solutions. With increasing the concentration, the three relaxation modes retarded, due to the hydrodynamic interaction. In addition, the topological interaction also retarded the orientation mode. The complex modulus of the tightly entangled region was separated into the component moduli using the strain-optical coefficient and the molecular theory. The curvature stress contributed to the rubbery plateau modulus in the tightly entangled region, as predicted by the Morse theory for the entangled systems. However, the relaxation time of curvature stress was shorter than the theoretical prediction, which is based on the fixed tube model. We speculate that the constraint release accelerates the relaxation of curvature stress but has a little effect on orientational stress." @default.
• W4200191539 created "2021-12-31" @default.
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• W4200191539 date "2021-12-07" @default.
• W4200191539 modified "2023-10-01" @default.
• W4200191539 title "Linear Viscoelasticity and Birefringence of Poly-γ-Benzyl-<scp>l</scp>-Glutamate Solutions" @default.
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• W4200191539 doi "https://doi.org/10.1021/acs.macromol.1c01398" @default.
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