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• W4200195944 abstract "Infrared nonlinear optical (IR NLO) materials are significant in laser technology for civil and military uses. Here, we report the synthesis, structural chemistry and NLO properties of a halogen-rich chalcohalide Sn7 Br10 S2 . Its noncentrosymmetric (NCS, P63 ) structure can be considered as partially aliovalent anion substitution of SnBr2 (P63 /m) induced centrosymmetric (CS) to NCS structural transformation. The 3D ∞ [Sn(1)6 Sn(2)6 Br6 X6 ]6- (X=Br/S) channel framework consists of Sn(1)BrX2 and Sn(2)X3 trigonal pyramids. It exhibits excellent NLO performance, including a strong phase-matchable NLO response of 1.5 × AgGaS2 and high laser-induced damage threshold of 6.3 × AgGaS2 .Investigation of the structure-NLO performance relationship confirms that the effective arrangement of Sn(1)BrX2 and Sn(2)X3 units predominantly contributes to the large SHG response. These results indicate Sn7 Br10 S2 is a potential IR NLO candidate and provides a new feasible system for promising NLO materials." @default.
• W4200195944 created "2021-12-31" @default.
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• W4200195944 date "2022-01-17" @default.
• W4200195944 modified "2023-10-18" @default.
• W4200195944 title "Sn ₇ Br ₁₀ S ₂ : The First Ternary Halogen‐Rich Chalcohalide Exhibiting a Chiral Structure and Pronounced Nonlinear Optical Properties" @default.
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• W4200195944 doi "https://doi.org/10.1002/anie.202115871" @default.
• W4200195944 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34951094" @default.
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