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- W4200202207 abstract "Sunlight is an abundant and clean energy source, the harvesting of which could make a significant contribution to society's increasing energy demands. Metal halide perovskites (MHP) have recently received attention for solar fuel generation through photocatalysis and solar-driven electrocatalysis. However, MHP photocatalysis is limited by low solar energy conversion efficiency, poor stability, and impractical reaction conditions. Compared to photocatalysis, MHP solar-driven electrocatalysis not only exhibits higher solar conversion efficiency but also is more stable when operating under practical reaction conditions. In this Perspective, we outline three leading types of MHP solar-driven electrocatalysis device technologies now in the research spotlight, namely, (1) photovoltaic-electrochemical (PV-EC), (2) photovoltaic-photoelectrochemical (PV-PEC), and (3) photoelectrochemical (PEC) approaches for solar-to-fuel reactions, including water-splitting and the CO2 reduction reaction. In addition, we compare each technology to show their relative technical advantages and limitations and highlight promising research directions for the rapidly emerging scientific field of MHP-based solar-driven electrocatalysis." @default.
- W4200202207 created "2021-12-31" @default.
- W4200202207 creator A5014185371 @default.
- W4200202207 creator A5030085518 @default.
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- W4200202207 creator A5078485962 @default.
- W4200202207 date "2021-12-27" @default.
- W4200202207 modified "2023-10-17" @default.
- W4200202207 title "Solar-to-Chemical Fuel Conversion via Metal Halide Perovskite Solar-Driven Electrocatalysis" @default.
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