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- W4200258958 abstract "Electrocatalytic nitrogen reduction reaction (NRR) at ambient conditions is a promising route for ammonia (NH3) synthesis but still suffers from low activity and selectivity. Here, ultrafine Sn nanoparticles (NPs) grown on carbon blacks (SnSC/C) have been synthesized through a wet-chemical method using sodium citrate dehydrate as a stabilizing agent. Benefiting from the small sizes of Sn NPs, the SnSC/C catalyst exhibits excellent electrocatalytic performance for NRR with a high Faradaic efficiency of 22.76% and an NH3 yield rate of 17.28 μg h-1 mg-1 in the 0.1 M Na2SO4 electrolyte, outperforming many reported electrocatalysts for NRR under similar conditions. Density functional theory calculation results reveal that the potential-determining step on Sn NPs is the generation of NHNH* through simultaneous hydrogenation of N2* by a H* and a H+/e- pair via Langmuir-Hinshelwood plus Eley-Rideal mechanisms." @default.
- W4200258958 created "2021-12-31" @default.
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- W4200258958 date "2021-12-13" @default.
- W4200258958 modified "2023-10-16" @default.
- W4200258958 title "Efficient Electrocatalytic Nitrogen Reduction to Ammonia on Ultrafine Sn Nanoparticles" @default.
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- W4200258958 doi "https://doi.org/10.1021/acsami.1c15324" @default.
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