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- W4200306575 abstract "The most efficient light-harvesting antennae found in nature, chlorosomes, are molecular tubular aggregates (TMAs) assembled by pigments without protein scaffolds. Here, we discuss a classification of chlorosomes as a unique tubular plastic crystal and we attribute the robust energy transfer in chlorosomes to this unique nature. To systematically study the role of supramolecular tube chirality by molecular simulation, a role that has remained unresolved, we share a protocol for generating realistic tubes at atomic resolution. We find that both the optical and the mechanical behavior are strongly dependent on chirality. The optical-chirality relation enables a direct interpretation of experimental spectra in terms of overall tube chirality. The mechanical response shows that the overall chirality regulates the hardness of the tube and provides a new characteristic for relating chlorosomes to distinct chirality. Our protocol also applies to other TMA systems and will inspire other systematic studies beyond lattice models." @default.
- W4200306575 created "2021-12-31" @default.
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- W4200306575 date "2022-01-01" @default.
- W4200306575 modified "2023-10-15" @default.
- W4200306575 title "The role of chirality and plastic crystallinity in the optical and mechanical properties of chlorosomes" @default.
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- W4200306575 doi "https://doi.org/10.1016/j.isci.2021.103618" @default.
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