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- W4200324824 abstract "We describe here reactions in which a carbonyl oxygen atom initiates cascade reactions by nucleophilic attack on a covalently attached benzyne. The benzynes are produced by thermal cyclization of triynes via hexadehydro-Diels-Alder reaction. The initially produced oxocarbenium/aryl carbanionic zwitterion is protonated in situ by an external protic nucleophile (NuH) of appropriate acidity. The resulting ion pair (oxocarbenium+/Nu-) collapses through several different mechanistic manifolds, adding to the diversity of structural classes that can be generated." @default.
- W4200324824 created "2021-12-31" @default.
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- W4200324824 date "2021-12-27" @default.
- W4200324824 modified "2023-09-23" @default.
- W4200324824 title "Trapping Reactions of Benzynes Initiated by Intramolecular Nucleophilic Addition of a Carbonyl Oxygen to the Electrophilic Aryne" @default.
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- W4200324824 doi "https://doi.org/10.1021/acs.orglett.1c04110" @default.
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